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Li Pre-Doping into Si Negative Electrodes Using Li-Naphthalenide Solutions with Various Ether Solvents For Next-Generation Batteries
2022
Journal of the Electrochemical Society
Four ethers were compared as solvents of lithium naphthalenide (Li-NTL) solutions to pre-dope Li into Si electrodes. The solvents of the Li-NTL solutions affected the stability and equilibrium potential (V eq). X-ray diffraction, thermodynamic characterization and ultraviolet-visible (UV–vis) spectroscopy were used to clarify the effects of the solvation structure, the lowest unoccupied molecular orbital (LUMO) energy of the solvent molecule and the ion pair structure between Li+ ions and
doi:10.1149/1945-7111/ac7673
fatcat:3hxjf6mzq5bwzgx2j4mgj4o7zm