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Intense green-emitting LiYF4:Ce,Tb tetragonal bipyramidal nanophosphors are synthesized and the composition is applied to bright dual-mode-emitting core/double-shell nanophosphors with a tetragonal bipyramidal morphology. The core/double-shell structure is directly confirmed by energy dispersive X-ray spectroscopy.doi:10.1039/c5nr05722a pmid:26729043 fatcat:qsavytzmdjhc7atlcgjeh4p6lu