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Transform-limited-pulse representation of excitation with natural incoherent light
2016
Journal of Chemical Physics
We study the natural excitation of molecular systems, applicable to, for example, photosynthetic light-harvesting complexes, by natural incoherent light. In contrast with the conventional classical models, we show that the light need not have random character to properly represent the resultant linear excitation. Rather, thermal excitation can be interpreted as a collection of individual events resulting from the system's interaction with individual, deterministic pulsed realizations that
doi:10.1063/1.4940028
pmid:26827198
fatcat:abuhfxbkgzfidbntjblmpwjhbi