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Generalized quantum Fokker-Planck equation for photoinduced nonequilibrium processes with positive definiteness condition
2016
Journal of Chemical Physics
This work provides a detailed derivation of a generalized quantum Fokker-Planck equation (GQFPE) appropriate for photo-induced quantum dynamical processes. The path integral method pioneered by Caldeira and Leggett (CL) [Caldeira and Leggett, Physica A 121, 587 (1983)] is extended for a nonequilibrium influence functional, which has been obtained for general cases where the ground and the excited electronic state baths can be different. Both nonequilibrium and non-Markovian effects are
doi:10.1063/1.4952477
pmid:27276940
fatcat:3uiftrzkzbeihnnvss5klkueke