Loss of spin glass behavior in ultrathin AuFe films

H. Fritzsche, J. M. van der Knaap, M. B. S. Hesselberth, G. J. Nieuwenhuys
2010 Physical Review B  
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more » ... n der Knaap, J. M.; Hesselberth, M. B. S.; Nieuwenhuys, G. J. https://publications-cnrc.canada.ca/fra/droits L'accès à ce site Web et l'utilisation de son contenu sont assujettis aux conditions présentées dans le site We determined the temperature dependence of the magnetization of thin Au 97 Fe 3 films in the thickness range between 1 and 50 nm by performing polarized neutron reflectivity measurements in a magnetic field of 6 T in a temperature range from 200 down to 2 K. For the films in the thickness range from 50 to 2 nm, we observed a Brillouin-type behavior of noninteracting Fe atoms down to 50 K followed by a strong reduction compared to the Brillouin curve below 50 K. This reduction in the magnetization is a measure of the spin glass frustration and depends on the film thickness below 20 nm as shown in our previous study ͓M. Saoudi, H. Fritzsche, G. J. Nieuwenhuys, and M. B. S. Hesselberth, Phys. Rev. Lett. 100, 057204 ͑2008͔͒ on Au 97 Fe 3 films. The present study is a continuation of this work extending the thickness range down to 1 nm. It shows that below 10 nm, the reduction in the spin glass magnetization compared to a Brillouin-type behavior decreases with decreasing film thickness. Finally, the magnetization of the 1-nm-thick film could be described with a Brillouin function also below 50 K proving that ultrathin Au 97 Fe 3 layers below 1 nm do not show spin glass behavior anymore but are paramagnetic.
doi:10.1103/physrevb.81.132402 fatcat:t6yxcpdunngqxlisxk4vsaoogu