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Composition and temperature dependence of the Raman spectra of the molten LnU-CsI (Ln= Ce, Dy, Ho) mixtures have been measured. The changes of the vibrational modes upon melting the polycrystalline compounds CS3L11I6 and Cs3Dy2l9 have also been measured. The spectral data suggest that, as for other LnX3-AX (Ln: lanthanide, A: alkali, X: F, Cl, Br) binaries, the six-fold coordination around the lanthanide is preserved at all compositions, including pure LnH melts, where a loose network-likedoi:10.1149/200424.0825pv fatcat:6wgmeowoh5hqhb6thh6i7yrwni