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Intramolecular Electron Transfer of CytochromecModified withN,N,N′,N″,N″-Diethylenetriaminepentaacetatocobaltate(III)
2003
Bulletin of the Chemical Society of Japan
Horse heart cytochrome c (cytc) modified with an N,N,N 0 ,N 00 ,N 00 -diethylenetriaminepentaacetatocobaltate(c) ion, [cytc c {Co c (dtpa)}], was prepared and characterized. The major component of singly modified [cytc c {Co c (dtpa)}] contains a [Co c (dtpa)] ion at Lys13, of which the "-amino group is linked with a carboxylate ion of dtpa. A oneelectron reduced protein, [cytc b {Co c (dtpa)}], was prepared by reduction with a methylviologen-radical cation, which was produced in situ by a
doi:10.1246/bcsj.76.1323
fatcat:tavrq2djuzaillbgdmcxug2yja