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Measuring the complex recombination dipole of aligned CO2molecules in high-order harmonic generation
2009
UVX 2008 - 9e Colloque sur les Sources Cohérentes et Incohérentes UV, VUV et X : Applications et Développements Récents
unpublished
Preserved Fulltext
We generate high order harmonics in aligned CO 2 molecules and measure the spectral amplitudes and phases as a function of the alignment angle. We control the quantum interference occurring in the recombination of an ultrafast laser-driven electron wavepacket with the highest occupied molecular orbital of CO 2 . By comparing to the emission of the reference system krypton, we obtain an experimental measure of the complex recombination dipole matrix element between the CO 2 HOMO and a continuum
doi:10.1051/uvx/2009011
fatcat:6v65xfh2bbcgbp5yfp4kmvvjjm