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Binary gas mixtures can be completely separated via dual-reflux pressure swing adsorption (DR-PSA) process, where pressure of the column to which the feed gas is supplied and the kind of gas employed for pressure swing determine different configurations. DR-PSA studies have been predominantly confined to the configurations that use heavy gas for pressure swing. For such configurations, we formerly reported an equilibrium theory-based optimum design approach that defined a complete separationdoi:10.1021/acs.iecr.8b04415.s001 fatcat:iiyl6edbsneehki2dge2shv5r4