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Localization of electronic wave packets in H2
2008
Journal of Physics B: Atomic, Molecular and Optical Physics
We demonstrate localization of electronic wave packets in the coupled channels of rotating and vibrating H 2 molecules using phase-shaped excitation pulses. The dynamics of Rydberg wave packets and their controlled preparation has been studied in detail in hydrogenic systems. We report here on a more general situation, where the strong channel couplings require full shaping of the optical phase, rather than a linear or quadratic chirp which is often sufficient in hydrogenic systems, or
doi:10.1088/0953-4075/41/7/074022
fatcat:jkj5rp4d3rdkvcdrt3tcomlrnm