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Time-resolved photoelectron imaging of S2 → S1 internal conversion in benzene and toluene
2011
Journal of Chemical Physics
Ultrafast internal conversion of benzene and toluene from the S 2 states was studied by time-resolved photoelectron imaging with a time resolution of 22 fs. Time−energy maps of the photoelectron intensity and the angular anisotropy were generated from a series of photoelectron images. The photoelectron kinetic energy distribution exhibits a rapid energy shift and intensity revival, which indicates nuclear motion on the S 2 adiabatic surface, while the ultrafast evolution of the angular
doi:10.1063/1.3586809
pmid:21568512
fatcat:7vcyr445nbddff4tzbb5a7xxre