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The influence of the pH on the synthesis of Zn(II) complexes derived from 1H-benzimidazol-2ylmethanamine (HL) has been investigated with X-ray crystallography, FAB mass spectrometry, NMR, infrared and Raman spectroscopy. The crystal structures of (1H-benzimidazol-2ylmethanamine)tetrachlorozincate( 2 -) dihydrogen [H 3 LZnCl 4 ] (2), (1H-benzimidazol-2ylmethanamine-κN 3 )trichlorozincate(1-) hydrogen hydrate [H 2 LZnCl 3 ]•H 2 O (3), (1Hbenzimidazol-2-ylmethanamine-κ 2 N 2 ,N 3 )dichlorozinc(II)doi:10.3998/ark.5550190.0009.514 fatcat:tj3zb4rrjzhr3gk6vwet4eqrgm