The cosmological moduli problem (CMP) comes in three parts: 1. potential violation of BBN constraints from late decaying moduli fields, 2. the moduli-induced gravitino problem wherein gravitinos are overproduced and 3. the moduli-induced lightest SUSY particle (LSP) overproduction problem. We examine the cosmological moduli problem and its connection to electroweak naturalness. We calculate the various two-body decay widths of a light modulus field into MSSM particles and gravitinos within

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... al supersymmetric models. We include both phase space and mixing effects. We examine cases without and with helicity suppression of modulus decays to gravitinos (cases 1 & 2) and/or gauginos (cases A & B). For case B1, we evaluate regions of gravitino mass m_{3/2} vs. modulus mass m_ϕparameter space constrained by BBN, by overproduction of gravitinos and by overproduction of neutralino dark matter, along with connections to naturalness. For this case, essentially all of parameter space is excluded unless m_ϕ>~ 2.5\times 10^3 TeV with m_ϕ<2m_{3/2}. For a potentially most propitious case B2 with ϕdecay to Higgs and matter turned off, then modulus branching fractions to SUSY and to gravitinos become highly suppressed at large m_ϕ. But since the modulus number density increases faster than the branching fractions decrease, there is still gross overproduction of neutralino dark matter. We also show that in this scenario the thermally produced gravitino problem is fixed by huge entropy dilution, but non-thermal gravitino production from moduli decay remains a huge problem unless it is kinematically suppressed with m_ϕ< 2m_{3/2}. In a pedagogical appendix, we present detailed calculations of modulus field two-body decay widths.