The present work details the design principles and field performance of software-augmented, multi-functional sensors capable of resolving solar spectral irradiance and atmospheric parameters, such as aerosol optical depth, total column ozone and precipitable water vapour. The primary motivation behind this research and development work is the solar industry's increasing need for spectral and atmospheric data, the acquisition of which, prior to this work, was not commercially practical or

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... fective. This thesis presents the direct solar spectral irradiance meter (SolarSIM-D2), which was designed for photovoltaic and atmospheric science applications. The instrument measures the direct normal irradiance (DNI) in six narrow wavelength bands. These measurements are combined with radiative transfer models to determine the spectral transmittance profiles of key atmospheric components, such as spectral aerosols, total column ozone and precipitable water vapour, and subsequently resolve the spectral DNI over the complete 280-4000 nm range. Multiple SolarSIM-D2s were calibrated and validated at the National Renewable Energy Laboratory (NREL) in the United States and at the World Radiation Center in Switzerland against reference instrumentation. In addition, a comprehensive uncertainty analysis was performed for all of the SolarSIM-D2's measurands. This work also describes the global solar spectral irradiance meter (SolarSIM-G), which was designed to resolve the spectral and broadband global irradiances over the complete 280-4000 nm spectral range, primarily for use in the photovoltaic industry. The all-sky parameterized transmittance model was developed, capable of deriving the spectral and broadband global irradiances from the SolarSIM-G's nine optical measurements under clear and cloudy conditions. This model uses radiative transfer algorithms to resolve in real-time the combined contribution of the direct and diffuse irradiance components, including the effects of atmospheric and cloud scattering. Multiple SolarSIM [...]