The anisotropy of small-scale temperature fluctuations in shear flows is analysed by making measurements in high-Reynolds-number atmospheric surface layers. A spherical harmonics representation of the moments of scalar increments is proposed, such that the isotropic part corresponds to the index j = 0 and increasing degrees of anisotropy correspond to increasing j. The parity and angular dependence of the odd moments of the scalar increments show that the moments cannot contain any isotropic

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... t (j = 0), but can be satisfactorily represented by the lowest-order anisotropic term corresponding to j = 1. Thus, the skewnesses of scalar increments (and derivatives) are inherently anisotropic quantities, and are not suitable indicators of the tendency towards isotropy.