Crystal symmetry and high-magnetic-field specific heat ofSrCu2(BO3)2
G. A. Jorge, R. Stern, M. Jaime, N. Harrison, J. Bonča, S. El Shawish, C. D. Batista, H. A. Dabkowska, B. D. Gaulin
2005
Physical Review B
We report measurements of the specific heat of the quantum spin liquid system SrCu2(BO3)2 in continuous magnetic fields H of up to 33 T. The specific heat vs temperature at zero field shows an anomaly at 8 K, marking the opening of a gap in the spin singlet excitations. At fields H 12 T, we clearly see a second anomaly that shifts to lower temperatures as H is increased. We attribute its origin to single triplet excitations of the singlet dimer ground state. This conclusion is supported by
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... lations of the specific heat, which reproduce the experimental data, made using the finite temperature Lanczos method to solve a Shastry-Sutherland Hamiltonian including nearest and next-nearest neighbor Dzyaloshinsky-Moriya interactions. The parameters used to fit the data are the exchange constants J = 74 K and J'/J = 0.62, and the Dzyaloshinsky-Moriya coupling constants |D|=6.1K, and |D'|=2.2K.
doi:10.1103/physrevb.71.092403
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