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Second-order nonlinear optical properties of Mg-doped lithium niobate single crystals are quantitatively studied from the chemical bond viewpoint. The results show that the secondorder nonlinear optical response of Mg-doped LiNbO 3 single crystals at 1079 nm decreases linearly with increasing Mg concentration in the crystal. This linear correlation is quantitatively evaluated in the current work.doi:10.1088/0953-8984/12/28/320 fatcat:u47dd3utjvgeveisrh4c2yavau