Soot Scattering Measurements in the Visible and Near-Infrared Spectrum [report]

Jinyu Zhu, Mun Y. Choi, George W. Mulholland, Louis A. Gritzo
2000 unpublished
Scattering to extinction cross-section ratios, q se , were measured using the NIST Large Agglomerate Optics Facility for soot produced from ethene and acetylene laminar diffusion flames. Measurements were performed using light sources at 543.5 nm, 632.8 nm, and 856 nm. The average scattering to extinction cross-section ratios for these wavelengths are equal to 0.245, 0.195, and 0.195 for ethene and 0.311, 0.228, and 0.237 for acetylene. The 856 nm measurements represent the longest wavelength
more » ... ongest wavelength for which accurate scattering measurements have been performed for soot. The size distribution and fractal properties of the two soots were determined to assess the effects of limited acceptance angle range, finite size of the sensor, and departure from cosine response on the uncertainty in the measurement of q se . The expanded relative uncertainty (95% confidence level) was found to be ‫%6ע‬ at the two visible wavelengths and ‫%8ע‬ at 856 nm. Both the magnitude and wavelength dependence of q se for the present experiments are significantly different from those reported by Krishnan et al. [7] for overfire soot produced using a turbulent flame. The results are compared with the predictions of fractal optics. Report Documentation Page Form Approved OMB No. 0704-0188 Public reporting burden for the collection of information is estimated to average 1 hour per response, including the time for reviewing instructions, searching existing data sources, gathering and maintaining the data needed, and completing and reviewing the collection of information. Send comments regarding this burden estimate or any other aspect of this collection of information, including suggestions for reducing this burden, to Washington Headquarters Services, Directorate for Information Operations and Reports, 1215 Jefferson Davis Highway, Suite 1204, Arlington VA 22202-4302. Respondents should be aware that notwithstanding any other provision of law, no person shall be subject to a penalty for failing to comply with a collection of information if it does not display a currently valid OMB control number.
doi:10.21236/ada455427 fatcat:fmfel7itibbgrexopgizd64i6u