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The spin structure of quantum well states (QWSs) in threemonolayer-thick gold overlayers on W(110) and Mo(110) is studied experimentally by spin-and angle-resolved photoelectron spectroscopy and theoretically by ab initio calculations. The spin-orbit coupling effects manifest themselves differently in the spin structure of atomic-like d and delocalized sp QWSs depending on how strongly the states are influenced by the substrate. The QWSs of a d character show a strong spin polarization with andoi:10.1088/1367-2630/15/12/125014 fatcat:2p6rf4z77barlj4mfy5waqewyu