Magnetic Field Effect on Crossover Temperature from Non-Fermi Liquid to Fermi Liquid Behavior in f2-Impurity Systems with Crystalline-Electric-Field Singlet State Competing with Kondo–Yosida Singlet State

Shinya Nishiyama, Kazumasa Miyake
2011 Journal of the Physical Society of Japan  
We investigate the magnetic field dependence of the physical properties of f^2-configuration systems with a crystalline-electric field (CEF) singlet ground state, which gives rise to a non- Fermi liquid (NFL) fixed point due to the competition between the Kondo-Yosida singlet and CEF singlet states. On the basis of the numerical renormalization group method, we find that the magnetic field breaks this NFL fixed point via two mechanisms: one causing the polarization of f-electrons and the other
more » ... iving the "channel" anisotropy. These two mechanisms induce a difference in the magnetic field dependence of the characteristic temperature T_F^*(H), the crossover temperature from NFL to Fermi-liquid behavior. While the polarization of f-electrons gives T_F^*(H) ∝ H^x (x∼2.0), the "channel" anisotropy gives the H-independent T_F^*(H). These two mechanisms cross over continuously at approximately the crossover magnetic field H_c, where an anomalous H-dependence of T_F^*(H) appears. Such T_F^*(H) well reproduces the NFL behaviors observed in Th_1-xU_xRu_2Si_2. We also find that the H-dependence of the resistivity and the magnetic susceptibility are in good agreement with the experimental results of this material. These results suggest that the NFL behaviors observed in Th_1-xU_xRu_2Si_2 can be understood if this material is located in the CEF singlet side near the critical phase boundary between the two singlet states.
doi:10.1143/jpsj.80.124706 fatcat:hk5jhejo5nawtj2vhvovabzlae