Frequency-domain infrared photothermal radiometry is introduced as a dynamic dental diagnostic tool and its main features are compared with modulated laser luminescence for quantifying sound and carious enamel or dentin. Dental caries found in the fissures or grooves of teeth is very difficult to diagnose or quantify with the present clinical techniques. Visual examination and dental radiographs do not detect the presence of decay until there has been significant carious destruction of the

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... . A high-spatial-resolution dynamic experimental imaging set-up, which can provide simultaneous measurements of laser-induced frequency-domain infrared photothermal radiometric and luminescence signals from defects in teeth, was developed. 1 Following optical absorption of laser photons, the new set-up can monitor simultaneously and independently the non-radiative (optical-to-thermal) conversion (infrared photothermal radiometry), and the radiative de-excitation (luminescence emission) in turbid media such as hard dental tissue. This work is intended to show the complementarity between modulated luminescence and photothermal frequency scans in detecting carious lesions in teeth. A sound extracted molar with a dentin-enamel interface was introduced to examine the depth profilometric abilities of the method. Occlusal surfaces of teeth with potential areas of demineralization or carious destruction in the fissures were examined and compared to the signals produced by the sound enamel establishing the depth profilometric abilities of the method. The significance to clinical dentistry lies in the potential of this technique to detect and monitor early carious lesions in the pits and fissures of teeth. Keywords: dental infrared photothermal radiometry, photothermal imaging and luminescence, carious teeth, pit and fissure caries, diagnosis of dental caries