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Publication costs assisfed by Bell Laboratories A computer simulation of the urban troposphere in northern New Jersey based on a chemistry of 143 reactions in 76 species has been performed without using any steady state approximations. After the fact, certain steady state relationships have been tested. The "photostationary state" relationship among NO, NOz, and O3 is found to be valid, but the free-radical HO-, which plays a vital part in the photochemistry of the troposphere, is shown to godoi:10.1021/j100540a026 fatcat:jbqfp2xqjzeojdxtuahpbm3ypq