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TbxGd1−xScO3 and TbxDy1−xScO3 solid-solution single crystals were grown by the Czochralski method to validate the practicality of solid solutions between neighboring RE scandates (REScO3). Within this material family, it is demonstrated that fine-tuning the pseudo-cubic lattice parameters between nearly all endmembers is now possible by adjusting the chemical composition of the mixed crystals. Film-tailored substrate lattice spacings enable fine adjustments of epitaxial strain or the growth ofdoi:10.26092/elib/15 fatcat:pvzsiq52fzhvref6ryrkc2hsie