In inhomogeneity and emission characteristics of InGaN

Yoichi Kawakami, Kunimichi Omae, Akio Kaneta, Koichi Okamoto, Yukio Narukawa, Takashi Mukai, Shigeo Fujita
2001 Journal of Physics: Condensed Matter  
Recombination dynamics of spontaneous and stimulated emissions have been assessed in InGaN-based light emitting diodes (LEDs) and laser diodes (LDs), by employing time-resolved photoluminescence and pump and probe spectroscopy. As for an In 0.02 Ga 0.98 N ultraviolet LED, excitons are weakly localized by 15 meV at low temperature, but they become almost free at room temperature (RT). It was found that addition of a small amount of In results in the reduction of nonradiative recombination
more » ... originating from point defects. The internal electric field does exist in InGaN active layers, and induces a large modification of excitonic transitions. However, it alone does not explain the feature of spontaneous emission observed in an In 0.3 Ga 0.7 N blue LED such as an anomalous temperature dependence of peak energy, almost temperature independence of radiative lifetimes and mobilityedge type behaviour, indicating an important role of exciton localization. The lasing mechanism was investigated for In 0.1 Ga 0.9 N near ultraviolet (390 nm), In 0.2 Ga 0.8 N violet-blue (420 nm) and In 0.3 Ga 0.7 N blue (440 nm) LDs. The optical gain was contributed from the nearly delocalized states (the lowest quantized levels (LQLs) within quantum wells) in the violet LD, while it was from highly localized levels with respect to the LQL by 250 meV for the violetblue LD, and by 500 meV for the blue LD. It was found that the photo-generated carriers rapidly (less than 1 ps) transferred to the LQL, and then relaxed to the localized tail within the timescale of a few ps, giving rise to the optical gain. Such gain spectra were saturated and other bands appeared in the vicinity of the LQL under higher photo-excitation.
doi:10.1088/0953-8984/13/32/308 fatcat:kjyilthyczdixj7fadcixa3hli