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Electrochemical nitrate (NO3−) reduction reaction (NO3−RR) represents an ideal alternative for ammonia (NH3) generation. Despite recent success on the synthesis of Cu-based electrocatalysts, the kinetics of Cu-catalyzed NO3−RR is still greatly limited by the slow proton transfer rate since the large energy barrier for water dissociation. Here, we report the construction of a yolk-shell structure, comprising a Cu core and Cu2Se shell that functions like the tandem nanoreactor. Specific, thedoi:10.21203/rs.3.rs-1006532/v1 fatcat:2s3svvubg5aobam5lxxchmjnre