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Quantitative Study of Enantiomer-Specific State Transfer
2022
We here report on a quantitative study of enantiomer-specific state transfer, performed in a pulsed, supersonic molecular beam. The chiral molecule 1-indanol is cooled to low rotational temperatures (1-2 K) and a selected rotational level in the electronic and vibrational ground state of the most abundant conformer is depleted via optical pumping on the S_{1}←S_{0} transition. Further downstream, three consecutive microwave pulses with mutually perpendicular polarizations and with a
doi:10.1103/physrevlett.128.173001
pmid:35570421
fatcat:onzezjvhnvdczlb4wv53ytutmm