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The role of electron spin resonance in the study of both natural and synthetic diamond is reviewed in this article. A brief survey of the physical significance of the constants in the spin Hamiltonian, as well as experimental technique, is given. The review then deals in some detail with the various nitrogen centres found in diamond, treating exchange-interaction, Jahn-Teller and relaxation effects associated with these centres. Acceptor impurities and transition-ion impurities are brieflydoi:10.1088/0034-4885/41/8/002 fatcat:5ontunz6ubcv5ayvbcreb25mce