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A theory of the intramolecular contributions to the broadening of the r(XH) absorption bands of hydrogen-bonded species is proposed, which is able to describe both vibrational predissociation and the formation of sum and difference bands. A formal method is developed for finding the wavefunctions and complex energy eigenvalues of quasi-stationary excited vibrational states of a linear triatomic system with realistic interactions. The theory is ap plied to the Me2O.HCl system. I t is found th adoi:10.1098/rspa.1974.0044 fatcat:qnl4lu2vgvfwhcqjmx7tnvya34