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Key indicators: single-crystal X-ray study; T = 295 K; mean (C-C) = 0.004 Å; R factor = 0.047; wR factor = 0.111; data-to-parameter ratio = 17.7. In the title complex, [CuCl 2 (C 16 H 14 N 4 S 2 )] n , the Cu atom lies on a center of inversion and is bridged by two adjacent pyrimidine N atoms and two chloride counter-ions to give a square-planar coordination geometry. The bidentate thioether ligands link adjacent Cu atoms into an infinite chain. Experimental Crystal data [CuCl 2 (C 16 H 14 N 4doi:10.1107/s1600536807039967 fatcat:dvomkqqaonht5ib3fnwgyq2xvu