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A B S T R A C T To constrain the relatively uncertain anthropogenic impact on the organic aerosol load, radiocarbon analyses were performed on aerosol samples, collected year-round, at six non-urban sites including a maritime background and three remote mountain stations, lying on a west-east transect over Western Europe. From a crude three component model supported by TOC and levoglucosan filter data, the fossil fuel, biomass burning and biogenic TOC fraction are estimated, showing at alldoi:10.1111/j.1600-0889.2008.00379.x fatcat:r2iw6mmtzvevllas7v5t65oftm