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Long-range orientation correlation in dipolar liquids probed by hyper-Rayleigh scattering
Journal of Chemical Physics
Hyper-Rayleigh scattering (HRS) is sensitive to long-range molecular orientation correlation in isotropic liquids composed of dipolar molecules. The correlation functions that appear in the calculation of HRS mediated by the vector part of the first hyperpolarizability β are the same as the correlation functions for the homogeneous isotropic random vector fields that appear in the description of fluid turbulence. Recent experiments measuring the angle and polarization dependence of HRS fromdoi:10.1063/1.4931973 pmid:26450319 fatcat:4a4vmf3m55afxf7i5oiuvnenwi