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In this work, we address the nature of electrochemically induced charged states in conjugated polymers, their evolution as a function of electrochemical potential, and their coupling to their local environment by means of transient absorption and Raman spectroscopies synergistically performed in situ throughout the electrochemical doping process. In particular, we investigate the fundamental mechanism of electrochemical doping in an oligoether-functionalized 3,4-propylenedioxythiophene (ProDOT)doi:10.26434/chemrxiv.13063916 fatcat:p6s5cnw7rvg3deljv2dgiv5kp4