HAADF-STEM imaging with sub-angstrom probes: a full Bloch wave analysis

Y. Peng
2004 Journal of Electron Microscopy  
A full coherent Bloch wave calculation is presented to investigate highangle annular dark-field image formation for sub-angstrom probes in scanning transmission electron microscopy (STEM). With increasing illumination angle, the contribution of the 1s bound state increases to a maximum at an optimum probe angle, after which we find increasing contributions from high-angle plane wave states around the periphery of the objective aperture. Examination of image contributions from different depths
more » ... thin a crystal shows an oscillatory behavior due to the beating between 1s and non-1s states. The oscillation period reduces with decreasing probe size, while the relative contribution from a specific depth increases. This signifies a changeover from a projection mode of imaging to a depth-slicing mode of imaging. This new mode appears capable of resolving threedimensional atomic structures in future generation aberration-corrected STEM.
doi:10.1093/jmicro/53.3.257 pmid:15332652 fatcat:hao6eh5dcjh47a2s5xgng3rdtm