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The density of reactive levels in NO2 unimolecular decomposition
1994
Journal of Chemical Physics
Laser induced fluorescence spectra of expansion-cooled NO*/Ne samples (I and 2 K) are reported for transitions that originate from the lowest rovibronic levels and terminate on levels near D,. At 1 K, nearly all transitions originate from N"=O. With the present resolution of 0.02 cm-', the 1 K spectra are resolved rather well. The high density of transitions is due to couplings between rovibronic levels with different N and K quantum numbers and with electronic characters that borrow oscillator
doi:10.1063/1.467403
fatcat:xqsbvfgzgjcoha6hbyqtopqjpy