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Analysis of pore size distributions based on crystalline representations of metal-organic frameworks (MOFs) featuring hierarchical pore systems, DUT-32, DUT-75, UMCM-1 and NU-1000, is presented here and leveraged to understand gas adsorption in these unique pore structures. Statistical analysis was used to effectively partition the pore space into distinct regions labelled by the pore size. This pore description was used to discover how adsorbates are located, with respect to the differentdoi:10.26434/chemrxiv-2022-ls3rp fatcat:vqnltoyqqrerjmkf5a6m5ciiqi