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It is eager to develop high-performance and cheap bifunctional electrochemical catalysts for both of the ORR or OER for the energy crisis and environmental problems. Herein, we report a series of ZIFderived Co-P-C co-doped polyhedral materials with a well-defined morphology. The optimized catalyst Co/P/MOFs-CNTs-700 exhibited favorable electrochemical activities with the lowest over potential of 420 mV to achieve the current density of 10 mA cm -2 for OER and the half potential of 0.8 V for ORRdoi:10.21203/rs.3.rs-17338/v1 fatcat:pd7vkh4m5jejtavort67cw3z6i