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Three new multi-step one-pot processes for high-yielding cyclohexanecarbonitrile synthesis starting from cyclohexanone were developed for industrial application. In contrast to the current synthetic process, all of the processes described were designed to proceed completely in methanol as a uniform solvent and the key oxidation step can be realized either as stoichiometric or catalytic. Atom efficiency of processes is relatively advanced with high regioselectivity, reaction by-products aredoi:10.4236/gsc.2014.42011 fatcat:s4bhno3uovakjph26iqxsbtosa