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4-N,N-dimethylamino-4′-N′-methyl-stilbazolium tosylate (DAST) organic single crystals controlled by (Z)-Octadec-9-enoic acid (oleic acid, OA) was grown by a slow-cooling method. The as-grown DAST single crystals were systematically characterized by FTIR, X-ray diffraction, second harmonic generation, and UV-vis spectroscopy. Results indicate that addition of OA into the DAST solutions leads to the controlled growth of DAST single crystals and consequently, the crystal quality and opticaldoi:10.3390/cryst9100494 fatcat:bxtgikwujnhf3c6qq5oemmk4iq