Aerosol Light Absorption at 1064 nm: Pollution Sources, Meteorological Parameters and Gas Pollutants in Qingdao Coastal Area, China release_kz7jy2ly35dxfaugb2eoc7nvwe

by Jie Chen, Wenyue Zhu, Qiang Liu, Xianmei Qian, Xuebin Li, Jianjie Zheng, Tao Yang, Qiuyi Xu

Published in Atmosphere by MDPI AG.

2021   Volume 12, Issue 12, p1553

Abstract

A two-month sampling campaign was carried out from 1 November to 30 December 2019, to investigate the light absorption of aerosols at coastal sites in Qingdao. The average values and standard deviations of the absorption coefficient (OAC) at λ = 1064 nm during the measurement period were 18.52 ± 13.31 Mm−1. Combined with the backward trajectory model, the aerosol absorption coefficient and gas pollution concentration of six possible air mass trajectories were obtained and calculated. The maximum absorption coefficient of local air masses was approximately 20.4 Mm−1 and anthropogenic pollution originated from mainly local sources in the Jiaozhou area. In our measurements at this site, the results also showed that there was a positive correlation between relative humidity (RH) and aerosol absorption. Without considering other factors, the size of aerosol particles grew with the increasing of RH, which changed the nonlinear relationship between the size and the absorption cross section of aerosol particles subsequently. In addition, the correlations between gas pollutants and OAC were calculated. The atmospheric environment is complex in sea–land intersection areas, especially in coastal cities. Analysis of various aerosol sources, meteorological conditions, and gas precursors enhances the study of aerosol optical absorption.
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