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The effect of Gd on trityl-based dynamic nuclear polarisation in solids
release_2ahvydgsyndzbor4kud4iejqfq
by
Enrico Ravera,
Daphna Shimon,
Akiva Feintuch,
Daniella Goldfarb,
Shimon Vega,
Alessandra Flori,
Claudio Luchinat,
Luca Menichetti,
Giacomo Parigi
Published
in Physical Chemistry, Chemical Physics - PCCP
by Royal Society of Chemistry (RSC).
2015 Volume 17, Issue 40, p26969-26978
Abstract
The increase in <sup>13</sup>C polarisation of <sup>13</sup>C-urea dissolved in samples containing water/DMSO mixtures and trityl radical (OX063) in the presence of Gd<sup>3+</sup> is explained by changes in electron relaxation, electron spectral diffusion and effective electron–proton hyperfine interaction.
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